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Can I enter Croatia from Austria with a single-entry Schengen visa by bus, and then return to Vienna by bus ?

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No.

Croatia is outside the Schengen area. They do accept dual and multiple entry Schengen Visas but not single entry ones.

http://www.mvep.hr/en/consular-information/visas/visa-requirements-overview/

  • i will enter by bus from vienna not by plane – bassel zaki Jul 28 '17 at 12:28
  • @basselzaki Doesn't matter, see my answer – Crazydre Jul 28 '17 at 13:09
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As stated in Timatic, the database used by airlines

Visa required, except for passengers with a double or multiple entry C visa issued by a Schengen Member State valid for all Schengen Member States and valid for the period of intended stay. They are visa exempt for a maximum stay of 90 days

So only double and multiple visas are valid, and it does not matter if you travel by bus, train, ship or plane. Meaning, you need a separate Croatian visa

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